Electron-vibration interaction in the presence of a switchable Kondo resonance realized in a molecular junction
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Autor:
D. Rakhmilevitch, R. Korytar, A. Bagrets, F. Evers, O. Tal
- Quelle:
- Datum: 2014
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The interaction of individual electrons with vibrations has been extensively studied. However,
the nature of the electron-vibration interaction in the presence of many-body electron correlation
such as a Kondo state has not been fully investigated. Here, we present transport measurements
on a Copper-phthalocyanine molecule, suspended between two silver electrodes in a break-junction
setup. Our measurements reveal both zero-bias and satellite conductance peaks, which are identifi ed
as Kondo resonances with a similar Kondo temperature. The relation of the satellite peaks to
electron-vibration interaction is corroborated using several independent spectroscopic indications,
as well as ab-initio calculations. Further analysis reveals that the contribution of vibration-induced
inelastic current is significant in the presence of a Kondo resonance.